The elementary excitations of magnets are called spin waves, and their corresponding quasi-particles are known as magnons. The rapidly growing field of Magnonics aims at using them as information... Show moreThe elementary excitations of magnets are called spin waves, and their corresponding quasi-particles are known as magnons. The rapidly growing field of Magnonics aims at using them as information carriers in a new generation of electronic devices, (almost) free of electric currents. Encoding information in the amplitude and/or phase of these coherent waves could lead to a drastic decrease in dissipated power, typically related to the motion of electrons ("Joule" or "Ohmic" heating).This dissertation describes the development and use of a new technique to study spin waves. This technique uses the electronic spins associated with nitrogen-vacancy (NV) centers as magnetic field sensors. An NV center is a light-emitting defect in the crystal lattice of diamond. Remarkably, the brightness of its emission depends on its spin state, sensitive to magnetic fields. This way, magnetic information can be investigated optically. Show less
Bertelli, I.; Simon, B.G.; Yu, T.; Aarts, J.; Bauer, G.E.W.; Blanter, Y.M.; Sar, T. van der 2021
Spin waves in magnetic insulators are low-damping signal carriers that can enable a new generation of spintronic devices. The excitation, control, and detection of spin waves by metal electrodes is... Show moreSpin waves in magnetic insulators are low-damping signal carriers that can enable a new generation of spintronic devices. The excitation, control, and detection of spin waves by metal electrodes is crucial for interfacing these devices to electrical circuits. As such, it is important to understand metal-induced damping of spin-wave transport, but characterizing this process requires access to the underlying magnetic films. Here it is shown that electronic sensor spins in diamond enable imaging of spin waves that propagate underneath metals in magnetic insulators. This capability is then used to reveal a 100-fold metal-induced increase in spin-wave damping. The damping enhancement is attributed to spin-wave-induced electrical currents as well as, above a certain frequency, three-magnon scattering processes. This interpretation is supported by deriving expressions for the current-induced damping and the three-magnon threshold from the Landau-Lifshitz-Gilbert equation that agree well with the observations. The detection of buried scattering centers further highlights the technique's power for assessing spintronic device quality. These results open new avenues for studying metal - spin-wave interactions and provide access to interfacial processes such as spin-wave injection via the spin-Hall effect. Show less
Simon, B.G.; Kurdi, S.; H. la; Bertelli, I.; Carmiggelt, J.J.; Ruf, M.; ... ; Sar, T. van der 2021
Controlling magnon densities in magnetic materials enables driving spin transport in magnonic devices. We demonstrate the creation of large, out-of-equilibrium magnon densities in a thin-film... Show moreControlling magnon densities in magnetic materials enables driving spin transport in magnonic devices. We demonstrate the creation of large, out-of-equilibrium magnon densities in a thin-film magnetic insulator via microwave excitation of coherent spin waves and subsequent multimagnon scattering. We image both the coherent spin waves and the resulting incoherent magnon gas using scanning-probe magnetometry based on electron spins in diamond. We find that the gas extends unidirectionally over hundreds of micrometers from the excitation stripline. Surprisingly, the gas density far exceeds that expected for a boson system following a Bose-Einstein distribution with a maximum value of the chemical potential. We characterize the momentum distribution of the gas by measuring the nanoscale spatial decay of the magnetic stray fields. Our results show that driving coherent spin waves leads to a strong out-of-equilibrium occupation of the spin-wave band, opening new possibilities for controlling spin transport and magnetic dynamics in target directions. Show less
Nava Antonio, G.; Bertelli, I.; Simon, B.G.; Medapalli, R.; Afanasiev, D.; Sar, T. van der 2021
We present a theory for quantum impurity relaxometry of magnons in thin films, exhibiting quantitative agreement with recent experiments without needing arbitrary scale factors used in theoretical... Show moreWe present a theory for quantum impurity relaxometry of magnons in thin films, exhibiting quantitative agreement with recent experiments without needing arbitrary scale factors used in theoretical models thus far. Our theory reveals that chiral coupling between prototypical spin >1/2 quantum impurities and magnons plays a central role in determining impurity relaxation, which is further corroborated by our experiments on nickel films interfaced with nitrogen-vacancy centers. Along with advancing magnonics and understanding decoherence in hybrid quantum platforms with magnets, the ability of a quantum impurity spin to sense chiral magnetic noise presents an opportunity to probe chiral phenomena in condensed matter. Show less
Bertelli, I.; Carmiggelt, J.J.; Yu, T.; Simon, B.G.; Pothoven, C.C.; Bauer, G.E.W.; ... ; Sar, T. van der 2020
Spin waves—the elementary excitations of magnetic materials—are prime candidate signal carriers for low-dissipation information processing. Being able to image coherent spin-wave transport is... Show moreSpin waves—the elementary excitations of magnetic materials—are prime candidate signal carriers for low-dissipation information processing. Being able to image coherent spin-wave transport is crucial for developing interference-based spin-wave devices. We introduce magnetic resonance imaging of the microwave magnetic stray fields that are generated by spin waves as a new approach for imaging coherent spin-wave transport. We realize this approach using a dense layer of electronic sensor spins in a diamond chip, which combines the ability to detect small magnetic fields with a sensitivity to their polarization. Focusing on a thin-film magnetic insulator, we quantify spin-wave amplitudes, visualize spin-wave dispersion and interference, and demonstrate time-domain measurements of spin-wave packets. We theoretically explain the observed anisotropic spin-wave patterns in terms of chiral spin-wave excitation and stray-field coupling to the sensor spins. Our results pave the way for probing spin waves in atomically thin magnets, even when embedded between opaque materials. Show less